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Can't believe that the orginal Texas Chain Saw Massacre has only been mentioned once in this thread. A very, very unsetlling film. Not jump scares really, just a constant feeling of dread and hopelessness throughout. Also, the very fact that someone could make a film filled with so much despair and "nastiness" is pretty grim too.
Other scary films in my opinion -The Shining, Silent Hill, IT, The Grudge (remake), Event Horizon,